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• W2007190775 abstract "Time-resolved fluorescence spectra of gas-phase toluene upon picosecond excitation at 266 nm were investigated as a function of temperature (296–1074 K) and bath gas composition (varying amounts of N2, O2, and CO2) at 1 bar total pressure with a temporal resolution of 50 ps. In the investigated temperature range the effective fluorescence lifetime drops with increasing temperature from 46 ± 3 ns to 0.05 ± 0.01 ns in N2 and CO2. In the presence of O2 at constant temperature the lifetimes also decrease significantly (e.g., from 46 ± 3 ns without O2 to 0.63 ± 0.05 ns in air at room temperature), whereas lifetimes are independent on the CO2 concentration. The implications of the results for the existing phenomenological model of predicting temporally integrated fluorescence intensities in toluene [W. Koban, J.D. Koch, R.K. Hanson, C. Schulz, Appl. Phys. B 80 (2005) 777] are discussed." @default.
• W2007190775 created "2016-06-24" @default.
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• W2007190775 date "2011-05-01" @default.
• W2007190775 modified "2023-09-25" @default.
• W2007190775 title "Temperature and bath gas composition dependence of effective fluorescence lifetimes of toluene excited at 266 nm" @default.
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• W2007190775 doi "https://doi.org/10.1016/j.chemphys.2011.03.013" @default.
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