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• W2007204595 abstract "We have studied the balance between olefin insertion and β-hydrogen transfer to monomer for all “well-defined” aluminum polymerization catalysts reported to date. Consistently, the balance is predicted to be significantly worse than for Me2AlEt, implying that none of the proposed active species should give a high-molecular-mass polymer. A more systematic analysis of ligand effects allows a rationalization of these results and shows that small modifications to the proposed active species are unlikely to solve the problem. We conclude that olefin polymerization at a single aluminum center is rather unlikely. Alternative interpretations of the experimental data are discussed." @default.
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• W2007204595 date "2001-10-01" @default.
• W2007204595 modified "2023-10-16" @default.
• W2007204595 title "Olefin Polymerization at Aluminum? A Theoretical Study" @default.
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• W2007204595 doi "https://doi.org/10.1021/om010696k" @default.
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