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• W2007205026 abstract "Studies of the vibration-vibration (VV) exchange in CO molecules excited up to vibration quantum numbers v = 20 have been performed both theoretically and experimentally. A new kinetic model which takes into account the multi-quantum VV exchange in the temperature range T = 100-300 K is described for the first time. A description is given of the experimental methodology allowing for studies of the effects of the relaxation of the vibrational distribution after a sudden disturbance. The disturbance of the vibrational distribution is produced by a Q-switched short pulse of single line radiation in fundamental band. The relaxation is studied by measuring the laser pulse energy of the second pulse initiated by resonator Q-switching produced with a variable time delay relative to the first pulse. A set of kinetic rate constants accepted in the model for various gas temperatures, vibration level numbers and number of exchanged vibration quanta from 1 to 4 is presented. The good agreement between the experimental data and the results of the advanced theory is the first direct evidence in support of the multi-quantum exchange model." @default.
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• W2007205026 date "2001-07-04" @default.
• W2007205026 modified "2023-10-18" @default.
• W2007205026 title "Theoretical modelling and experimental studies of the multi-quantum vibration exchange in vibrationally excited CO molecules" @default.
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• W2007205026 doi "https://doi.org/10.1088/0022-3727/34/14/319" @default.
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