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- W2007292041 abstract "A novel supramolecular clipping design for influencing the photophysical properties of functional molecular assemblies, by the preorganization (clipping) of chromophores, is described. Several chromophores end functionalized with molecular recognition units were designed. These molecular recognition units serve as handles to appropriately position these systems upon noncovalent interactions with multivalent guest molecules (supramolecular clippers). Towards this goal, we have synthesized 1,5-dialkoxynaphthalene (DAN) and naphthalenediimide (NDI) functionalized with dipicolylethylenediamine (DPA) motifs. These molecules could preorganize upon noncovalent clipping with adenosine di- or triphosphates, which resulted in preassociated excimers and mixed (cofacial) charge-transfer (CT) assemblies. Chiral guest binding could also induce supramolecular chirality, not only into the individual chromophoric assembly but also into the heteromeric CT organization, as seen from the strong circular dichroism (CD) signal of the CT transition. The unique ability of this design to influence the intermolecular interactions by changing the binding strength of the clippers furthermore makes it very attractive for controlling the bimolecular photophysical processes." @default.
- W2007292041 created "2016-06-24" @default.
- W2007292041 creator A5038142574 @default.
- W2007292041 creator A5054930574 @default.
- W2007292041 creator A5079095437 @default.
- W2007292041 date "2014-03-12" @default.
- W2007292041 modified "2023-09-23" @default.
- W2007292041 title "Supramolecular Clippers for Controlling Photophysical Processes through Preorganized Chromophores" @default.
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- W2007292041 doi "https://doi.org/10.1002/chem.201304106" @default.
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