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• W2007352214 startingPage "A1107" @default.
• W2007352214 abstract "Layered sodium-ion cathode material P2-Na0.85Li0.17Ni0.21Mn0.64O2 was investigated using operando XAS to characterize structural changes occurring in the material during electrochemical sodiation/desodiation. Based on XANES data, the primary mode of charge compensation in this material is due to Ni2–3/4+ redox activity, while the Mn remains in the +4 oxidation state, thereby providing stability to this material during extended cycling. Investigation of the initial state of the compound by high resolution synchrotron XRD and 6Li MAS NMR revealed a significant amount of structural disorder due to integration of a small amount of monoclinic layered Li phase within the overall hexagonal layered Na-structure, which manifests as Li-induced stacking faults. High quality EXAFS data could be obtained using our cell construction and revealed the local structural evolution around the redox active Ni centers." @default.
• W2007352214 created "2016-06-24" @default.
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• W2007352214 date "2014-01-01" @default.
• W2007352214 modified "2023-09-25" @default.
• W2007352214 title "Operando Structural Characterization of the Lithium-Substituted Layered Sodium-Ion Cathode Material P2-Na_0.85Li_0.17Ni_0.21Mn_0.64O₂by X-ray Absorption Spectroscopy" @default.
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• W2007352214 doi "https://doi.org/10.1149/2.088406jes" @default.
• W2007352214 hasPublicationYear "2014" @default.
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