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- W2007357108 abstract "An interference quenching of the ${ensuremath{nu}}^{ensuremath{'}ensuremath{'}}=1$ vibrational line in the resonant Auger decay of N $1sensuremath{rightarrow}{ensuremath{pi}}^{*}$ core-excited ${mathrm{N}}_{2}$ is observed and analyzed. The intensity ratio between the ${ensuremath{nu}}^{ensuremath{'}ensuremath{'}}=1$ and ${ensuremath{nu}}^{ensuremath{'}ensuremath{'}}=0$ vibrational levels of the ${mathrm{X}}^{2}{ensuremath{Sigma}}_{g}^{+}$ final state shows a surprising nonmonotonous variation as a function of frequency detuning, going through a minimum with a complete suppression of ${ensuremath{nu}}^{ensuremath{'}ensuremath{'}}=1$. We have developed a simple model which shows a linear relation between the value of the detuning frequency for this minimum and the equilibrium bond distance ${R}_{c}^{0}$ of the core-excited state. A new way is thus established of determining the equilibrium bond distance for the core-excited state with a precision $ensuremath{delta}{R}_{c}^{0}<{10}^{ensuremath{-}3}text{ }text{ }AA{}$." @default.
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- W2007357108 date "2002-08-16" @default.
- W2007357108 modified "2023-09-29" @default.
- W2007357108 title "Interference Quenching ofν′′=1Vibrational Line in Resonant Photoemission ofN2: A Possibility to Obtain Geometrical Information on the Core-Excited State" @default.
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- W2007357108 doi "https://doi.org/10.1103/physrevlett.89.103002" @default.
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