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- W2007440018 abstract "Abstract Rhodium–phosphite catalysts were found to effectively mediate double‐bond migrations within unsaturated esters. Once the double‐bond is in conjugation with the carboxylate group, they also catalyze the Michael addition of carbon and nitrogen nucleophiles. In the presence of these catalysts, unsaturated carboxylates enter a dynamic equilibrium of positional and geometrical double‐bond isomers. The conjugated species are continuously removed through 1,4‐additions with formation of β‐amino esters or β‐arylated products, depending on the nucleophile employed. The applicability of both protocols to a range of substrates, such as fatty esters of different chain lengths and double‐bond positions, and several nucleophiles including arylborates and primary and secondary amines, is demonstrated." @default.
- W2007440018 created "2016-06-24" @default.
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- W2007440018 creator A5071663387 @default.
- W2007440018 creator A5086344136 @default.
- W2007440018 date "2011-07-15" @default.
- W2007440018 modified "2023-10-18" @default.
- W2007440018 title "Regioselective Synthesis of β-Aryl- and β-Amino-Substituted Aliphatic Esters by Rhodium-Catalyzed Tandem Double-Bond Migration/Conjugate Addition" @default.
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- W2007440018 doi "https://doi.org/10.1002/chem.201100654" @default.
- W2007440018 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21766361" @default.
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