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• W2007448369 abstract "The matrix formula developed in the context of hetrochain theory, Mw = Mwp + WF(I − M)−1S, was applied to describe the molecular weight development during free-radical homopolymerization. All of the required probabilistic parameters are expressed in terms of the kinetic-rate constants and various concentrations. In free-radical polymerization, the primary chains are formed consecutively, and the number of heterochain types, N, is extrapolated to infinity. Practically, such extrapolation can be conducted on the basis of the calculated values for only three different N values with sufficient accuracy. This matrix formula is valid regardless of the chemical and reactor systems used, as long as the primary chain-connection statistics is considered Markovian. The gel point can be determined simply by solving an equation det(I − M) = 0. © 2004 Wiley Periodicals, Inc. J Polym Sci Part B: Polym Phys 42: 2791–2800, 2004" @default.
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• W2007448369 date "2004-01-01" @default.
• W2007448369 modified "2023-09-27" @default.
• W2007448369 title "Heterochain model for simultaneous long-chain branching and crosslinking. II. Application to free-radical polymerization" @default.
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• W2007448369 doi "https://doi.org/10.1002/polb.10534" @default.
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