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- W2007473332 abstract "In atomic-layer deposition (ALD), organoaluminum as trimethyl-aluminum (TMA) on a freshly molecular beam epitaxy grown In0.20Ga0.80As(001)-4 × 2 surface has three forms: Al bonding with 1, 2, and 3 methyl groups. The ALD method of using one pulse (0.1 s) of TMA plus one pulse (0.1 s) of water was ineffective in passivating the surface, as demonstrated by the increased intensity of the reacted surface components with high numbers of pulses. The intact TMA was physisorbed on the trough In atoms, while the methyl-deficient precursors are either bridged with two As atoms or on the row-edge As atoms. After the water pulse on the TMA-covered surface, a bond in the bridged As atoms was scissored off to produce the As-Al-CH3 and As-OH, and the physisorbed TMA was unaffected. TMA removed some row In atoms, which allowed the In and Ga atoms in the second layer to form OH bonds after the water exposure. The appearance of the As-OH bonds may cause interfacial defect density (Dit) a peak at the midgap." @default.
- W2007473332 created "2016-06-24" @default.
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- W2007473332 date "2013-05-28" @default.
- W2007473332 modified "2023-09-26" @default.
- W2007473332 title "Interfacial electronic structure of trimethyl-aluminum and water on an In<sub>0.20</sub>Ga<sub>0.80</sub>As(001)-4 × 2 surface: A high-resolution core-level photoemission study" @default.
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- W2007473332 doi "https://doi.org/10.1063/1.4807400" @default.
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