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• W2007796021 abstract "We investigate DNA collisions with a small cylindrical obstacle using BD (Brownian dynamics) simulation and derive the mean hold-up time of hooked DNA molecules based on existing micromechanical models and observations of the present work. Recently, Randall and Doyle (Macromolecules 2006, 39, 7734) experimentally explored this DNA collision problem using single molecule microscopy and proposed a set of micromechanical models. They found that so-called X collisions, with increasing total extension during unhooking, are a dominant collision type. Our numerical simulations corroborate that the proportion of X collisions is much higher than that of other collision types for a wide range of Peclet numbers and molecular weights. We compare the predictions of the previously proposed micromechanical models to our simulation results. The derived expressions for the mean hold-up time are consistent with our simulation data and available experimental data for a wide range of Peclet numbers. It is expected that the derived mean hold-up time will be helpful in the design of separation devices using post arrays." @default.
• W2007796021 created "2016-06-24" @default.
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• W2007796021 date "2007-11-10" @default.
• W2007796021 modified "2023-09-26" @default.
• W2007796021 title "Brownian Dynamics Simulations of a DNA Molecule Colliding with a Small Cylindrical Post" @default.
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• W2007796021 doi "https://doi.org/10.1021/ma0710434" @default.
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