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• W2008064386 abstract "The effect of metal coordination of 2-(1-(9-anthryl)methyl-1,2,3-triazol-4-yl)-6-(1-n-octyl-1,2,3-triazol-4-yl)pyridine (2) on the emission of the appended anthryl group was investigated in acetonitrile. The tridentate 2,6-bis(1,2,3-triazol-4-yl)pyridyl ligand included in 2 is referred herein as ‘clickate’. Titrating zinc(II) perchlorate or zinc(II) chloride into the solution of fluorescent ligand 2 results in quenching, which is attributed to the formation of a dark 1:1 ZnII complex of 2. Frontier molecular orbital analysis and cyclic voltammetric data support the occurrence of photoinduced electron transfer from the excited state of the anthryl group to the ZnII-bound clickate moiety, which relaxes the excited fluorophore non-radiatively, i.e. quenches fluorescence. Fluorescence quenching of clickate 2 upon forming the PbII complex was also observed. The ZnII/PbII-coordination chemistry of clickate was characterised via X-ray crystallography, isothermal titration calorimetry, 1H NMR spectroscopy and absorption spectroscopy using the symmetrically substituted clickate 2,6-bis(1-n-octyl-1,2,3-triazol-4 yl)pyridine (1)." @default.
• W2008064386 created "2016-06-24" @default.
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• W2008064386 date "2012-06-19" @default.
• W2008064386 modified "2023-09-26" @default.
• W2008064386 title "Zn^II and Pb^II coordination chemistry of 2,6-bis(1,2,3-triazol-4-yl)pyridine (clickate) and the metal ion-dependent emission of ‘clickate’–appended anthracene" @default.
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• W2008064386 doi "https://doi.org/10.1080/10610278.2012.695790" @default.
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