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- W2008274301 abstract "Single molecules that act as light-energy transducers (e.g., converting the energy of a photon into atomic-level mechanical motion) are examples of minimal molecular devices. Here, we focus on a molecular switch designed by merging a conformationally locked diarylidene skeleton with a retinal-like Schiff base and capable of mimicking, in solution, different aspects of the transduction of the visual pigment Rhodopsin. Complementary ab initio multiconfigurational quantum chemistry-based computations and time-resolved spectroscopy are used to follow the light-induced isomerization of the switch in methanol. The results show that, similar to rhodopsin, the isomerization occurs on a 0.3-ps time scale and is followed by <10-ps cooling and solvation. The entire (2-photon-powered) switch cycle was traced by following the evolution of its infrared spectrum. These measurements indicate that a full cycle can be completed within 20 ps." @default.
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- W2008274301 date "2008-11-18" @default.
- W2008274301 modified "2023-10-18" @default.
- W2008274301 title "An artificial molecular switch that mimics the visual pigment and completes its photocycle in picoseconds" @default.
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- W2008274301 doi "https://doi.org/10.1073/pnas.0802376105" @default.
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