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- W2008331369 abstract "A system of planar rotators representing H 2 S and D 2 S molecules is investigated quantum-statistically, using the mean-field approximation based on an eight-sublattice model. The equilibrium molecular orientation is determined by competition among the dipole-dipole interaction between guest molecules, the host-guest interaction and the quantum kinetic energy. The system has a complex order parameter describing an average direction of dipoles. Both Rbar1 and Rbar3 structures and the effect of the depolarization field are studied. A comparison with experiment by use of theoretical phase diagrams gives: the low-temperature phase has the Rbar1 structure with an antiferroelectric order of dipoles; the direction and arrangement of dipoles in equilibrium for H 2 S significantly differ from those for D 2 S because of the quantum nature of the rotational motion." @default.
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- W2008331369 date "1994-02-15" @default.
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- W2008331369 title "Quantum Effects on the Orientational Ordering of H2S and D2S Molecules Enclosed in β-Quinol Clathrate" @default.
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- W2008331369 doi "https://doi.org/10.1143/jpsj.63.593" @default.
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