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- W2008695211 abstract "Semi-continuous analysers for ammonia and nitric acid have been constructed, using modifications to published designs. The ammonia analyser is based upon a diffusion scrubber, and that for nitric acid upon conversion of HNO3 to NO2 (via NO) and analysis by luminol chemiluminescence. Both have response times of around 5 min and detection limits of around 100 ppt. Comparison of the semi-continuous analysers with conventional filter pack and denuder procedures shows good agreement. The nitric acid analyser correlates extremely closely with the filter pack method, whilst the ammonia analyser is highly comparable with measurements made by annular denuder. Both instruments become less reliable at relative humidities above 90%. The instruments have been used to measure [NH3] [HNO3] concentration products at a site in suburban Birmingham. In general, these concentration products conform extremely well to values predicted from chemical thermodynamics for the equilibrium dissociation of pure ammonium nitrate. The exception is for measurements made at very high humidities, here it appears that kinetic constraints lead to a slow reaction and actual atmospheric concentration products appreaciably exceed equilibrium values." @default.
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- W2008695211 title "Validation of techniques for fast response measurement of HNO3 and NH3 and determination of the [NH3] [HNO3] concentration product" @default.
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- W2008695211 doi "https://doi.org/10.1016/1352-2310(94)90099-x" @default.
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