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- W2008755724 abstract "We present an effective four-level density matrix model for describing ultrafast interferometric three-photon photoemission (3PPE) from a metal surface. The model accounts for the slow resonant and the fast nonresonant excitation channels through the energy continua, in the presence of energy and phase relaxation of the electronic states. Calculations are presented for the case of a gold surface irradiated with $9.5phantom{rule{0.3em}{0ex}}mathrm{fs}$ Ti:sapphire laser pulses, where we find good agreement with recent experimental results for the photocharge vs the time delay between two identical laser subpulses. Numerical results are also presented for the photocurrent densities of the different excitation channels and the photocharge densities vs time delay for various laser pulse widths from 100 down to $2.5phantom{rule{0.3em}{0ex}}mathrm{fs}$ (one optical period). It is shown that interferometric 3PPE can be used to measure sub-$10text{ensuremath{-}}mathrm{fs}$ laser pulse widths and for extracting lifetimes of conduction electrons." @default.
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- W2008755724 date "2008-02-29" @default.
- W2008755724 modified "2023-10-14" @default.
- W2008755724 title "Modeling of ultrafast interferometric three-photon photoemission from a metal surface irradiated with sub-<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mn>10</mml:mn><mml:mtext>−</mml:mtext><mml:mi>fs</mml:mi></mml:mrow></mml:math>laser pulses" @default.
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- W2008755724 doi "https://doi.org/10.1103/physrevb.77.085436" @default.
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