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- W2009012124 abstract "Interfacial reactions between a sealing glass–ceramic and electrolyte present a challenge for the development of sealing materials. In this paper, we report for the first time, the interfacial reaction between Hf-containing borosilicate glass–ceramics and 8 mol.% yttria-stabilized zirconia (8YSZ) electrolyte. The results show that the interdiffusion between the glass–ceramics and the 8YSZ can be confined to a ∼2 μm zone at the interface. Additionally, the HfO2 dopant can inhibit the formation of monoclinic ZrO2 and zirconates in the reaction couples of glass–ceramics and 8YSZ, which can be attributed to the Hf-containing phase formation, e.g., Ca6Hf19O44 and Ca3HfSi2O9. Moreover, the formation of the Hf-containing phases contributes to a low conductivity of the glass–ceramics, e.g., 1.9 × 10−7 to 1.6 × 10−6 S cm−1 at 700 °C. These results demonstrate the suitability of the Hf-containing glass–ceramics as sealing materials for SOFC applications." @default.
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- W2009012124 date "2015-08-01" @default.
- W2009012124 modified "2023-10-14" @default.
- W2009012124 title "Reducing the interfacial reaction between borosilicate sealant and yttria-stabilized zirconia electrolyte by addition of HfO2" @default.
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- W2009012124 doi "https://doi.org/10.1016/j.jeurceramsoc.2015.02.010" @default.
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