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• W2009177712 abstract "In this paper, we report a novel all-carbon two-dimensionally ordered nanocomposite electrode system on the basis of the consideration of host−guest chemistry, which utilizes synergistic interactions between a nanostructured matrix of ordered mesoporous carbon (OMC) and an excellent electron acceptor of nanosized fullerene (C60) to facilitate heterogeneous electron-transfer processes. The integration of OMC-C60 by covalent interaction, especially its electrochemical applications for electrocatalysis, has not been explored thus far. Such integration may even appear to be counterintuitive because OMC and C60 provide opposite electrochemical benefits in terms of facilitating heterogeneous electron-transfer processes. Nevertheless, the present work demonstrates the integration of OMC and C60 can provide a remarkable synergistic augmentation of the current. To illuminate the concept, eight kinds of inorganic and organic electroactive compounds were employed to study the electrochemical response at an OMC-C60 modified glassy carbon (OMC-C60/GC) electrode for the first time, which shows more favorable electron-transfer kinetics than OMC/GC, carbon nanotube modified GC, C60/GC, and GC electrodes. Such electrocatalytic behavior at OMC-C60/GC electrode could be attributed to the unique physicochemical properties of OMC and C60, especially the unusual host−guest synergy of OMC-C60, which induced a substantial decrease in the overvoltage for NADH oxidation compared with GC electrode. The ability of OMC-C60 to promote electron transfer not only suggests a new platform for the development of dehydrogenase-based bioelectrochemical devices but also indicates a potential of OMC-C60 to be of a wide range of sensing applications because the electrocatalysis of different electroactive compounds at the OMC-C60/GC electrode in this work should be a good model for constructing a novel and promising electrochemical sensing platform for further electrochemical detection of other biomolecules." @default.
• W2009177712 created "2016-06-24" @default.
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• W2009177712 date "2008-05-14" @default.
• W2009177712 modified "2023-10-09" @default.
• W2009177712 title "Electrochemical Sensing Platform Based on the Highly Ordered Mesoporous Carbon−Fullerene System" @default.
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• W2009177712 doi "https://doi.org/10.1021/ac702496k" @default.
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