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- W2009229039 abstract "A kinetic study is conducted to investigate the elementary processes scheme that produces methane decomposition as a small percentage of this gas is introduced downstream in the flowing afterglow of a nitrogen microwave discharge. For this purpose a self-consistent kinetic model is used for the discharge and corresponding afterglow including, besides the species associated with active nitrogen, such as vibrationally excited molecules, and metastables and N(4S) atoms, various hydrocarbons formed from methane decomposition, and other species produced in nitrogen–methane reactions. It is observed that CH4 is primarily dissociated in CH3 and CH2 in collisions with N2(A), the stable hydrogen cyanide molecule HCN is formed at an intermediate stage of the process, HCN and CH2 give place to the formation of CN(X 2Σ+), and ultimately C atoms are produced by collisions of CN(X) with N atoms. The predicted concentrations so obtained are compared with experimental determinations of N and C atoms and of N2(B 3Πg) and CN(B 2Σ+) states, these latter obtained from spectroscopic measurements." @default.
- W2009229039 created "2016-06-24" @default.
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- W2009229039 creator A5088340380 @default.
- W2009229039 date "2007-06-04" @default.
- W2009229039 modified "2023-10-06" @default.
- W2009229039 title "Kinetic modelling of a N<sub>2</sub>flowing microwave discharge with CH<sub>4</sub>addition in the post-discharge for nitrocarburizing treatments" @default.
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- W2009229039 doi "https://doi.org/10.1088/0022-3727/40/12/011" @default.
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