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- W2009381846 abstract "In this paper, the mass transfer of CO2 into a reservoir brine sample is studied experimentally at high pressures and elevated temperatures. The equilibrium concentration of CO2 in the reservoir brine and the density of CO2-saturated brine are measured by saturating the brine with CO2. The mass-transfer rate of CO2 into the brine is determined by monitoring the pressure decay inside a closed, visual, high-pressure PVT cell. It is found that the density of the brine with dissolved CO2 increases linearly with CO2 concentration. As CO2 gradually dissolves into the brine by molecular diffusion, a concentration-induced density gradient is generated near the CO2−brine interface. Under the influence of gravity, this concentration-induced density gradient causes natural convection, which accelerates the mass-transfer rate of CO2 into the brine. The modified diffusion equation with an effective diffusivity is applied to model the mass-transfer process. It is found that the determined effective diffusivities of CO2..." @default.
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- W2009381846 date "2005-10-06" @default.
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- W2009381846 title "Accelerated Mass Transfer of CO<sub>2</sub> in Reservoir Brine Due to Density-Driven Natural Convection at High Pressures and Elevated Temperatures" @default.
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- W2009381846 doi "https://doi.org/10.1021/ie050497r" @default.
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