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- W2009457592 abstract "Novel isotope effects were observed in desorption kinetics and adsorption geometry of cyclohexane on Rh(111) by the use of infrared reflection absorption spectroscopy, temperature programmed desorption, photoelectron spectroscopy, and spot-profile-analysis low energy electron diffraction. The desorption energy of deuterated cyclohexane (C6D12) is lower than that of C6H12. In addition, the work function change by adsorbed C6D12 is smaller than that by adsorbed C6H12. These results indicate that C6D12 has a shallower adsorption potential than C6H12 (vertical geometric isotope effect). The lateral geometric isotope effect was also observed in the two-dimensional cyclohexane superstructures as a result of the different repulsive interaction between interfacial dipoles. The observed isotope effects should be ascribed to the quantum nature of hydrogen involved in the C–H···metal interaction." @default.
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- W2009457592 date "2012-06-07" @default.
- W2009457592 modified "2023-10-04" @default.
- W2009457592 title "Kinetic and geometric isotope effects originating from different adsorption potential energy surfaces: Cyclohexane on Rh(111)" @default.
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- W2009457592 doi "https://doi.org/10.1063/1.4725714" @default.
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