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- W2009461611 abstract "The hindered motion and the structure of the CO2− radical adsorbed on various zeolites were investigated by means of ESR spectroscopy. The adsorbed CO2− radical was obtained by the γ-irradiation of zeolites with carbon dioxide labeled with 13C. The results show that the interaction of the CO2− radical with the zeolite surface changes with the electrostatic field on the surface. The motion and the structure of the adsorbed CO2− radical are affected by the properties of the zeolite surfaces; the former is also influenced by the extent of exchange of the cation on zeolite, regardless of the time of irradiation, before or after the introduction of carbon dioxide. The formation of the CO2− radical on zeolites was interpreted on the basis of such a mechanism that electrons are initially trapped by the surface of zeolite upon the irradiation and then transferred to carbon dioxide molecules. The results also show that the process of the electron transfer depends on the kind of cation." @default.
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- W2009461611 date "1972-11-01" @default.
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- W2009461611 title "Electron Spin Resonance Studies of the Carbon Dioxide Anion Radical Adsorbed on X-Type Zeolites" @default.
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- W2009461611 doi "https://doi.org/10.1246/bcsj.45.3362" @default.
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