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- W2009501825 abstract "Abstract The acid strength of solid acid materials can be assessed using the linear free energy relationship, applying the Hammett–Brown equation ( log k X / k H = ρ σ + ) for the H/D exchange with substituted benzenes. The magnitude of the ρ varies for different solid acid materials (Amberlyst-15, zeolite HUSY, K-10 montmorillonite, and niobic acid) and is associated with the degree of proton transfer in the transition state. The results were compared with the ρ values obtained for H/D exchange with sulfuric acid solutions, indicating that neither solid acid is stronger than 98% sulfuric acid solution. Calculations also revealed that H/D exchange is mostly concerted, with little degree of charge development in the aromatic ring in the transition state." @default.
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- W2009501825 date "2007-06-10" @default.
- W2009501825 modified "2023-10-17" @default.
- W2009501825 title "Assessing the acid strength of solid acid catalysts with the use of linear free energy relationship: H/D exchange with substituted benzene derivatives" @default.
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- W2009501825 doi "https://doi.org/10.1016/j.jcat.2007.03.012" @default.
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