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- W2009882569 abstract "The electropolymerization of methylthio-substituted oligothiophenes 2–4 has been studied. Theoretical and experimental results reveal that only 4,4′-disubstituted derivatives yield polymeric films. The reason for this is that electron-donating methylthio (=methylsulphonyl) substituents in the ‘outer’ β-positions of the starting compounds 2–4, which cause high spin densities at the corresponding α-C atoms, favour fast coupling steps between the reacting oligomers during all stages of the electropolymerization. All data clearly indicate that the electropolymerization of donor-substituted thiophenes is not a chain propagation process but a series of successive ‘dimerization’ steps. The resulting polymers have been characterized by voltammetric measurements, in situ conductivity experiments and spectroelectrochemistry." @default.
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- W2009882569 date "1998-07-01" @default.
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- W2009882569 title "β,β-Disubstituted oligothiophenes, a new oligomeric approach towards the synthesis of conducting polymers" @default.
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- W2009882569 doi "https://doi.org/10.1016/s0022-0728(98)00100-4" @default.
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