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- W2009898846 abstract "On the Knowledge of the Catalytic Dimerization of Acrylic Acid Derivatives by Palladium Complexes. III Reactions of β-Palladio Acrylates and Their Relation to the Catalytic Reaction Complexes of the type L2PdCl(CH CHCOOCH3) (L2 = 2 PPh3 or Ph2PCH2CH2PPh2) were decomposed to dimethyl muconate by pyrolysis or by substraction of the phosphine ligands with (CH3CN)2PdCl2 in acetonitrile. The last mentioned reaction gave Δ3-dimethyl dihydromuconate in the presence of hydrochloric acid. Δ3-Dimethyl dihydromuconate was also formed by decomposition of (Ph2PCH2CH2PPh2) PdCl (CH CHCOOCH3) with HBF4 in acetonitrile, but the analogous reaction in methyl acrylate as solvent gave Δ2-dimethyl dihydromuconate. Thus, we have simulated the formation of the two main products of the catalytic dimerization of methyl acrylate with palladium(II)chloride in a stoichiometric manner. Mechanisms with hydride and carbene intermediates are discussed." @default.
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- W2009898846 title "Zur Kenntnis der katalytischen Dimerisation von Acryls�urederivaten mit Hilfe von Palladium-Komplexen. III. Reaktionen von ?-Palladioacrylestern und deren Beziehung zur Katalytischen Reaktion" @default.
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- W2009898846 doi "https://doi.org/10.1002/prac.19803220514" @default.
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