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- W2009945596 abstract "The role of orbital polarization for ultrafast charge transfer between an atomic adsorbate and a substrate is explored. Core hole clock spectroscopy with linearly polarized x-ray radiation allows to selectively excite adsorbate resonance states with defined spatial orientation relative to the substrate surface. For c(4×2)S∕Ru(0001) the charge transfer times between the sulfur 2s−13p*+1 antibonding resonance and the ruthenium substrate have been studied, with the 2s electron excited into the 3p⊥* state along the surface normal and the 3p‖* state in the surface plane. The charge transfer times are determined as 0.18±0.07 and 0.84±0.23fs, respectively. This variation is the direct consequence of the different adsorbate-substrate orbital overlap." @default.
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- W2009945596 date "2007-11-06" @default.
- W2009945596 modified "2023-09-23" @default.
- W2009945596 title "Ultrafast charge transfer and atomic orbital polarization" @default.
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- W2009945596 doi "https://doi.org/10.1063/1.2781395" @default.
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