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- W2009968581 abstract "The interaction of state-selected and oriented N2O molecules in the first excited n2=1 bending mode with one monolayer of Cs on Pt(111) is studied by means of time-of-flight mass spectroscopy in a molecular beam experiment. State-selected and oriented N2O molecules were prepared using electrostatic hexapole and dipole fields. The emission of N2 molecules induced by the abstraction reaction (N2O+Cs→CsO+N2) depends strongly on the molecular state and its orientation. Direct abstraction and backscattering of N2 molecules is observed for N2O ground-state molecules in the n2=1 first vibrationally excited bending mode. A distinct steric effect has been found for N2 molecules emitted specularly with respect to the incoming N2O molecules. These findings are explained in a picture where direct N2 emission is triggered by resonant N2O ionization (harpooning). The results are discussed in the context of recent exoelectron emission experiments." @default.
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- W2009968581 date "1998-05-01" @default.
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- W2009968581 title "State- and orientation-dependent N2 emission in the N2O+Cs reaction" @default.
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- W2009968581 doi "https://doi.org/10.1016/s0039-6028(97)00954-0" @default.
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