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- W2010090243 abstract "PEG-based diblock and triblock copolymers bearing blocks of lipid-mimetic monomer units, 1,3-didodecyloxy-2-glycidyl-glycerol (DDGG), were synthesized via anionic polymerization. They were characterized by 1H nuclear magnetic resonance spectroscopy and gel permeation chromatography. The copolymers are of a higher poly(DDGG) to PEG ratio compared to related copolymers studied earlier. They self-associate both in aqueous (water) and nonaqueous (n-heptane) solutions. The self-assembled structures were studied by simultaneous dynamic and static light scattering. In both solvents nanoparticles with weight-average molecular weights reaching 390 × 106 were formed. Cryogenic transmission electron microscopy performed on aqueous dispersions revealed coexistence of unilamellar vesicles and fractions of multilamellar vesicles or vesicles with internal folded lamellar structures. On the basis of numerical calculations of the area per lipid anchor, formation of reversed vesicles and disks in heptane by the diblock and triblock copolymers, respectively, was suggested. The aggregates are able to solubilize large amounts of substances that are insoluble in the medium in which the aggregates are formed. At high heptane contents the close bilayer structure of the normal vesicles in water no longer exists. Upon the addition of water the dispersions of reverse vesicles or disks in heptane undergo transition from reverse bilayers to monolayer stabilized water-in-oil emulsions." @default.
- W2010090243 created "2016-06-24" @default.
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- W2010090243 date "2004-05-14" @default.
- W2010090243 modified "2023-09-25" @default.
- W2010090243 title "Formation of Normal and Reverse Bilayer Structures by Self-Assembly of Nonionic Block Copolymers Bearing Lipid-Mimetic Units" @default.
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- W2010090243 doi "https://doi.org/10.1021/jp0304576" @default.
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