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- W2010419212 abstract "Liquid-crystalline (LC) poly(3,3'''-didodecyl-quaterthiophene) (PQT-12) was investigated to optimize its side alkyl ordering and pi-conjugated structure for high performance organic field-effect transistor (OFET) applications. Initially, low-crystal films spun-cast on OTS-treated SiO2 substrates were further crystallized via either thermal or solvent treatments. At temperatures (125-138 degrees C) driving a LC state of PQT-12, mobile chains were better migrated into preformed crystals. The resulting films showed highly crystal nanofibrils, in which pi-conjugated polymer backbones (with an conjugated backbone spacing, d(010) of 3.80 A) and the orientation of self-assembled side-chains were tilted with respect to the film surface, respectively. However, via melting or solvent exposure providing isotropic states, film crystallization generated less ordered crystals with randomly oriented side-chains, increasing d(010) up to 4.16 A. As a result, the usage of LC characteristic allowed us to consistently achieve the desirable crystal structure of PQT-12 and to robustly obtain high field-effect mobility for FET applications." @default.
- W2010419212 created "2016-06-24" @default.
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- W2010419212 date "2012-02-01" @default.
- W2010419212 modified "2023-09-25" @default.
- W2010419212 title "Structural Control Over Self-Assembled Crystals of π-Conjugated Poly(3,3‴-didodecyl-quaterthiophene) for Organic Field-Effect Transistor Applications" @default.
- W2010419212 doi "https://doi.org/10.1166/jnn.2012.4578" @default.
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