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• W2010466958 abstract "Diagrammatic perturbation theory and the spherical tensor formalism are used to model the signal observed in time-resolved, two-colour resonant four-wave mixing (TC-RFWM). An analysis using the Liouville formalism illustrates how TC-RFWM can be used to perform state-selective quantum beat spectroscopy in three-level systems by suitably designing three experimental features: the excitation scheme for the matter-field interaction, the time ordering of the laser pulses and the polarization of the incident laser beams. In contrast to traditional fluorescence quantum beat spectroscopy, time-resolved TC-RFWM results in a background-free, coherent signal that allows for high-resolution detection of the spectrally unresolved energy structure within a selected material state of the three-level system. The beats are shown to result from the quantum interference between different Liouville-space pathways in the laser-induced evolution of the material density operator and appear as a temporal modulation in the amplitude of the light beam emerging as the output of the mixing process. This type of control of a coherent optical field, based on the selective preparation of superposition states, is reminiscent of other recently developed optical techniques such as coherent population trapping and lasing without inversion." @default.
• W2010466958 created "2016-06-24" @default.
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• W2010466958 date "1999-09-01" @default.
• W2010466958 modified "2023-09-27" @default.
• W2010466958 title "State-selective quantum beat spectroscopy via coherent control of Liouville-pathway interference in two-colour resonant four-wave mixing" @default.
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• W2010466958 doi "https://doi.org/10.1088/0953-4075/32/18/301" @default.
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