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- W2010477978 abstract "The EPR Technique has been used to investigate the isotopic exchange between oxygen from the adsorbed species and the oxygen from either the lattice or the gas phase. The reactions are as follows: (16O2-)s+17O2rightleftarrows(17O2-)s+16O2,g (17O2-)s+16Ol2-?(16O17O-)s+17Ol2- where the subscripts s, g and l refer to adsorbed, gaseous or lattice oxygen respectively. The hyperfine lines due to the nuclear spin (I=5/2) of 17O (in oxygen enriched to 58 atom% of 17O) have been used to monitor the isotopic exchange. The predicted behaviour of the different possible mechanisms is compared to the experimental results which show, on MgO, that reaction (1) is reversible and occurs via an (O4-)s intermediate. The possible geometries of such a species are compared and discussed. On the other hand, reaction (2) does not appear to be reversible and is favoured by UV or gamma irradiation." @default.
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- W2010477978 date "1974-01-01" @default.
- W2010477978 modified "2023-09-26" @default.
- W2010477978 title "EPR Studies of Isotopic Exchange Involving Adsorbed Oxygen Species on MgO" @default.
- W2010477978 doi "https://doi.org/10.7567/jjaps.2s2.a911a" @default.
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