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• W2010482355 abstract "The adsorption and diffusion of ferrocene (FC) in thin MOF films of type Cu2(ndc)2(dabco) were studied by X-ray diffraction and using a quartz-crystal microbalance (QCM) at different temperatures. A quantitative analysis of the uptake curves in the QCM during loading with FC from the gas phase yields 0.19 FC compounds per pore at a temperature of 305 K and of 0.06 at 335 K, respectively. From an analysis of this temperature dependence we obtain an adsorption enthalpy of -30 kJ mol(-1). A quantitative analysis of the time dependence of the QCM uptake curves yields very small diffusivities on the order of 10(-19) to 10(-17) m(2) s(-1), while the activation energy for diffusion amounts to +90 kJ mol(-1). These results show that using a quartz crystal microbalance for uptake studies in SURMOFs is a valuable tool for investigating very slowly diffusing compounds in nanoporous materials." @default.
• W2010482355 created "2016-06-24" @default.
• W2010482355 creator A5064307923 @default.
• W2010482355 creator A5082394369 @default.
• W2010482355 date "2013-01-01" @default.
• W2010482355 modified "2023-09-27" @default.
• W2010482355 title "Adsorption and diffusion in thin films of nanoporous metal–organic frameworks: ferrocene in SURMOF Cu2(ndc)2(dabco)" @default.
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• W2010482355 doi "https://doi.org/10.1039/c3cp50578b" @default.
• W2010482355 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23660829" @default.
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