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- W2011010992 abstract "Zinc(II) promotes the reduction of unactivated ketones and aldehydes by (methyl-substituted) 1-methyl-1,4-dihydropyridines. Coordination of the dihydropyridines to the metal, which occurs via their annular nitrogen atoms, is essential for hydrogen-transfer. The reductions proceed best in apolar non-aromatic solvents, which are unable to compete with the carbonyl group of the substrate for a coordination site at the metal. Virtually no hydrogen-transfer takes place in the absence of Zn(II) salts or when zinc coordination complexes are used in which the metal is coordinatively saturated.The results of this study are discussed in terms of a possible relationship with the role of zinc in alcohol dehydrogenases and metal-catalyzed reductions in biomimetic systems." @default.
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- W2011010992 date "2010-09-02" @default.
- W2011010992 modified "2023-09-26" @default.
- W2011010992 title "Zinc(II)-promoted reduction of ketones by 1-methyl-1,4-dihydropyridines" @default.
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- W2011010992 doi "https://doi.org/10.1002/recl.19800991006" @default.
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