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• W2011036815 abstract "Abstract The reactivity of alkyne- and vinylidene-substituted clusters towards molecular hydrogen in homogeneous conditions has been studied by means of GC and GC/MS techniques. The reactivity of the homo- and hetero-metallic cluster frames (containing nickel and one of the iron triad metals) is discussed, as well as that of the coordinated ligands. Under hydrogen the cluster cores are modified, sometimes as a part of a catalytic cycle. The products obtainable from the coordinated small molecules seem to depend mainly on the overall electronic situation of the clusters or on the CC distances in the alkynes, and to a lesser extent on the number of coordinating metal centres. In some instances it was observed that when both free alkynes and substituted clusters were present, only the coordinated alkynes were hydrogenated." @default.
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• W2011036815 date "1983-11-01" @default.
• W2011036815 modified "2023-09-27" @default.
• W2011036815 title "Metal clusters in catalysis. The reactivity of alkyne-and vinylidene-substituted homo- and hetero-metallic clusters towards molecular hydrogen in homogeneous conditions" @default.
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• W2011036815 doi "https://doi.org/10.1016/s0022-328x(00)99260-x" @default.
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