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- W2011041129 abstract "We present one-dimensional particle-in-cell simulations of multielectron dissociative ionization (MEDI) of diatomic and linear triatomic molecules exposed to an intense subpicosecond laser pulse. Our method allows us to deal with all the electrons and nuclei explicitly, and to follow the temporal evolution of MEDI. The simulation results confirm that ionization probability is strongly enhanced at a certain critical internuclear distance. This occurs when the internal potential barriers surpass the external one and electrons are localized in higher potential wells. The mechanism of enhanced ionization in a diatomic and a triatomic molecule can be understood in a similar way, though all three potential wells participate in it for the triatomic case. Nevertheless, the occurrence of ionization is not necessarily localized at the critical distance. In addition, our simulations show that there is no significant difference in the final charge state of ion fragments between diatomic and linear triatomic molecules. The relative smallness of the critical distance in our results may suggest that not only the ionization taking place preferably near the critical distance, but also the non-Coulombic nature of the molecular potential curves, cause the experimentally observed kinetic-energy defects." @default.
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- W2011041129 date "2000-05-10" @default.
- W2011041129 modified "2023-10-14" @default.
- W2011041129 title "Particle-in-cell simulations of multiple ionization of small molecules in a strong laser field" @default.
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- W2011041129 doi "https://doi.org/10.1103/physreva.61.063408" @default.
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