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- W2011069895 abstract "The catalytic properties of atomically precise, thiolate-protected Au38(SR)24 (R = CH2CH2Ph) nanoclusters supported on CeO2 were investigated for CO oxidation in a fixed bed quartz reactor. Oxygen (O2) thermal pretreatment of Au38(SR)24/CeO2 at a temperature between 100 and 175 °C largely enhanced the catalytic activity, while pretreatment at higher temperatures (>200 °C) for removing thiolate instead gave rise to a somewhat lower activity than that for 175 °C pretreatment, and the ligand-off clusters were also found to be less stable. The CO conversion in the case of wet feed-gas (i.e. the presence of H2O vapor) was appreciably higher than the case of dry feed-gas when the reaction temperature was kept relatively low (between 60 and 80 °C), and interestingly the ligand-on and ligand-off catalysts exhibited opposite response to water vapor. Finally, we discussed some insights into the catalytic reaction involving the well-defined gold nanocluster catalyst." @default.
- W2011069895 created "2016-06-24" @default.
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- W2011069895 date "2013-01-01" @default.
- W2011069895 modified "2023-10-14" @default.
- W2011069895 title "CeO2-supported Au38(SR)24 nanocluster catalysts for CO oxidation: a comparison of ligand-on and -off catalysts" @default.
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- W2011069895 doi "https://doi.org/10.1039/c3nr00970j" @default.
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