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- W2011094311 abstract "An atomic force microscopy (AFM) and confocal Raman microscopy study of the interfacial electron transfer of a dye-sensitization system, i.e., alizarin adsorbed upon TiO2 nanoparticles, has revealed the distribution of the mode-specific vibrational reorganization energies encompassing different local sites (∼250-nm spatial resolution). Our experimental results suggest inhomogeneous vibrational reorganization energy barriers and different Franck−Condon coupling factors of the interfacial electron transfer. The total vibrational reorganization energy was inhomogeneous from site to site; specifically, mode-specific analyses indicated that energy distributions were inhomogeneous for bridging normal modes and less inhomogeneous or homogeneous for nonbridging normal modes, especially for modes far away from the alizarin−TiO2 coupling hydroxyl modes. The results demonstrate a significant step forward in characterizing site-specific inhomogeneous interfacial charge-transfer dynamics." @default.
- W2011094311 created "2016-06-24" @default.
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- W2011094311 date "2005-07-28" @default.
- W2011094311 modified "2023-09-23" @default.
- W2011094311 title "Probing Inhomogeneous Vibrational Reorganization Energy Barriers of Interfacial Electron Transfer" @default.
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- W2011094311 doi "https://doi.org/10.1021/jp058043v" @default.
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