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- W2011109110 abstract "The photolysis of SO2 in H2 has been studied at 147 nm (xenon line) and at 116.5 – 123.6 nm (krypton lines). Chemiluminescent reactions of photofragments lead to the observation of the fluorescence of SO2 (xenon lamp), OH(A → X) emission (xenon and krypton lamps), S2(B → X) and SO(B → X) radiative transitions (krypton lamp). The SO(A → X) emission observed with the krypton lamp is attributed to the photodissociation of SO2 at 116.5 nm (second krypton line). The phosphorescence (a → X) of SO2, and not its fluorescence, is obtained only on irradiation with the krypton lamp and it is interpreted as the result of internal conversion from the excited state (singlet or more probably triplet) to the emitting first triplet state. The quantum yield for SO3 formation is shown to be Π ⩽ 0.4 at 123.6 nm. The primary photodissociation processes giving S(1D or 3P) + O2 are more important with krypton lines than with the xenon line." @default.
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- W2011109110 date "1975-03-01" @default.
- W2011109110 modified "2023-09-25" @default.
- W2011109110 title "Photochemistry of SO2 in the vacuum—U.V. II. Luminescence studies" @default.
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- W2011109110 doi "https://doi.org/10.1016/0047-2670(75)85029-5" @default.
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