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• W2011126075 abstract "The temperature dependence of the rate constants for the reactions of ground-state atomic nitrogen with halogens were measured by means of a pulse radiolysis-resonance absorption technique. The rate constants for iodine and bromine were well expressed by the following Arrhenius expressions below 410 K: k(N+I2)=1.1×106 exp(−1170/T); k(N+Br2)=1.1×105 exp(−1490/T), in units of m3 mol−1 s−1. The rate constant for the reaction with chlorine was found to be 1.1×103 m3 mol−1 s−1 at 411 K. Below this temperature, the rate constants for N+Cl2 were too small to be measured. The preexponential factors for the I2 and Br2 reactions were found to be much smaller than the semiempirically calculated ones. These small preexponential factors suggest that the reactions between N(4S) and halogens proceed via nonadiabatic routes." @default.
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• W2011126075 date "1986-12-01" @default.
• W2011126075 modified "2023-09-26" @default.
• W2011126075 title "The Arrhenius Parameters for the Reactions of N(2⁴S_3⁄2) with Halogen Molecules" @default.
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• W2011126075 doi "https://doi.org/10.1246/bcsj.59.3755" @default.
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