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• W2011187906 abstract "ABSTRACT The all-trans to 13-cis isomerization of the retinal chromophore in bacteriorhodopsin (bR) plays an essentialrole in Nature (e.g., in photosynthesis of halobacteria). bR is a candidate for optical nanodevices driven by laserpulses, and a prospective material for optical memory storage devices and photoswitches. 1 From the viewpointof possible applications of bR in nanodevices we performed an experimental study of the isomerization yield byexcitation with tailored laser pulses, using a coherent control approach. 2 With specially shaped excitation pulses(found in optimization experiments) we are able to manipulate the 13-cis yield in bR over an absolute range of60 % (30% enhancement as well as 30% suppression in comparison to excitation with a transform-limited pulse)while keeping the absorbed excitation energy at a constant level.Keywords: coherence, coherent control, bacteriorhodopsin, FROG, isomerization, pump-probe, protein, retinal 1. INTRODUCTION The photo-isomerization of the retinal molecule contained in rhodopsins results in the appearance of a long-lived isomer ( all-trans in rhodopsin and 13-cis in bR). This light-driven photoreaction can be used for dierentphotonic nano-devices, based on rhodopsins. For example, very recently a symbiosis of a cell membrane containingbR and a nanotube network transistor was demonstrated." @default.
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• W2011187906 date "2005-09-28" @default.
• W2011187906 modified "2023-09-23" @default.
• W2011187906 title "Optimal control of the isomerization yield in bacteriorhodopsin using tailored light pulses" @default.
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• W2011187906 doi "https://doi.org/10.1117/12.629963" @default.
• W2011187906 hasPublicationYear "2005" @default.
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