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• W2011205155 abstract "A systematic study of cobalt site preferences has been carried out in a number of rare-earth iron compounds. The Mossbauer source technique employed in this work offers a direct and unambiguous way to determine quantitatively cobalt site preferences in these compounds at extremely low cobalt contents. Data quality as well as counting efficiency for the source ${(}^{57}$Co doped) samples is improved by using a resonant-conversion-electron detector. Our results have produced convincing evidence that cobalt substitutes preferentially for iron in all of the compounds investigated. We find that the site volume is the dominant factor controlling preferential cobalt substitutions at transition-metal sites with volume 12.2 A${mathrm{r{}}}^{3}$. The cobalt preference for a site decreases linearly with increasing site volume at a rate of ensuremath{sim}0.9 A${mathrm{r{}}}^{mathrm{ensuremath{-}}3}$. In general, cobalt shows a preference for sites with a volume greater than 11.8 A${mathrm{r{}}}^{3}$. As the site volume becomes sufficiently large (ensuremath{ge}12.2 A${mathrm{r{}}}^{3}$), the negative enthalpy of mixing between cobalt and rare earth plays a significant role and leads cobalt to prefer sites with the highest number of rare-earth nearest neighbors." @default.
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• W2011205155 date "1993-05-01" @default.
• W2011205155 modified "2023-10-16" @default.
• W2011205155 title "Cobalt site preferences in iron rare-earth-based compounds" @default.
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• W2011205155 doi "https://doi.org/10.1103/physrevb.47.11230" @default.
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