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- W2011515455 abstract "To investigate the supramolecular interactions of the mechanically interlocked rotaxane pendants and conjugated polymer backbones, four analogous polymers were systematically synthesized by copolymerization of a 9-alkylidene-9H-fluorene monomer with various monomers, which contained a diketopyrrolopyrrole unit tethered with a dumbbell unit, a metalated [2]rotaxane, a demetalated orthogonal H-bonded [2]rotaxane, and a simple alkyl chain, to furnish P1, P2, P3, and P4, respectively. Prevailing 1H NMR and UV–vis to NIR titration profiles indicated that the novel polyrotaxane P3 showed a sensitive and reversible acid–base molecular switch capability via supramolecular interactions in contrast to the other polymers (P1, P2, and P4). Compared with the other polymers, P3 possessed a narrower bandgap, which was also confirmed by the computational study. Prominently, the monitoring of a controllable nanoself-assembly process of P3 was obtained by reversible acid–base molecular switch approaches. The orthogonal H-bonded pendant [2]rotaxane unit and the steric demand of P3 judiciously allowed to morph into a hierarchical nanostructure via interconvertible H-bonds, anion−π and π–π stackings, and hydrophobic interactions." @default.
- W2011515455 created "2016-06-24" @default.
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- W2011515455 date "2013-08-23" @default.
- W2011515455 modified "2023-10-10" @default.
- W2011515455 title "An Acid–Base Controllable Hierarchical Nanostructure from a NIR-Absorbing Conjugated Polyrotaxane-Based Optical Molecular Switch" @default.
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- W2011515455 doi "https://doi.org/10.1021/ma401485b" @default.
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