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• W2011568314 abstract "According to the Gibbs-Thomson equation, the vapor pressure pr of clusters of radius r depends on the surface free energy σ. The latter is a function of the number of nearest neighbors of the surface atoms, Za. The decrease of Za with cluster size is discussed for several models of Wulff polyhedra. Based on the data for these models, a size dependent σr is introduced which results in pr, σ≫Pr and renders the Gibbs-Thomson equation increasingly inaccurate for r<30 A. The cluster shape as well as the mode of separation of atoms are affected by the presence of a surface. The consequences of introducing σr and, possibly, a size dependent Ωr into classical nucleation theory are discussed. It is concluded that the atomistic theory describes more reliably the formation of nuclei consisting of only a few atoms." @default.
• W2011568314 created "2016-06-24" @default.
• W2011568314 creator A5034515259 @default.
• W2011568314 date "1971-06-01" @default.
• W2011568314 modified "2023-09-23" @default.
• W2011568314 title "The enhanced vapor pressure of small clusters" @default.
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• W2011568314 doi "https://doi.org/10.1016/0040-6090(71)90038-1" @default.
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