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- W2011589962 abstract "We present a multifrequency electron spin resonance study in the range of 4--420 GHz of the quasi-one-dimensional, nondimerized, quarter-filled Mott insulators, $ensuremath{delta}text{ensuremath{-}}{({text{EDT-TTF-CONMe}}_{2})}_{2}X$ $(X={text{AsF}}_{6},text{Br})$. In the high-temperature orthorhombic phase above $Tensuremath{sim}190text{ }text{K}$, the magnitude and the temperature dependence of the high-temperature spin susceptibility are described by a $S=frac{1}{2}$ Heisenberg antiferromagnetic chain with ${J}_{{text{AsF}}_{6}}=298text{ }text{K}$ and ${J}_{text{Br}}=474text{ }text{K}$ coupling constants for $X={text{AsF}}_{6}$ and Br, respectively. We estimate from the temperature dependence of the linewidth $(ensuremath{Delta}H)$ an exchange anisotropy, ${J}^{ensuremath{'}}/J$ of $ensuremath{sim}2ifmmodetimeselsetexttimesfi{}{10}^{ensuremath{-}3}$. The frequency dependence of $ensuremath{Delta}H$ and the $g$ shift have an unusual quadratic dependence in all crystallographic orientations that we attribute to an antisymmetric exchange (Dzyaloshinskii-Moriya) interaction." @default.
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- W2011589962 date "2010-06-29" @default.
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- W2011589962 title "Spin dynamics in the<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi>S</mml:mi><mml:mo>=</mml:mo><mml:mstyle scriptlevel=1><mml:mfrac bevelled=false><mml:mn>1</mml:mn><mml:mn>2</mml:mn></mml:mfrac></mml:mstyle></mml:mrow></mml:math>antiferromagnetic chain compounds<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi>δ</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mrow><…" @default.
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- W2011589962 doi "https://doi.org/10.1103/physrevb.81.224438" @default.
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