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- W2011794324 abstract "We have performed quantum mechanical scattering calculations on the collinear H+H2 reaction on the Porter-Karplus potential energy surface at energies in the vicinity of the two lowest energy resonances. From the scattering matrices obtained, we have calculated the eigenvalues and eigenvectors of Smith's collision lifetime matrix. The eigenvalues of the collision lifetime matrix provide an unambiguous means for characterizing the resonances, as only one eigenvalue of the matrix undergoes rapid variation with energy in the neighborhood of the resonance. The two resonances are found to be located at 0.875 and 1.310 eV total energy, and have widths (fwhm in the collision lifetime versus energy curves) of 0.021 and 0.028 eV and lifetimes of 91 and 85 fs, respectively. Consideration of the energy dependence of the components of the eigenvectors of the collision lifetime matrix shows that although both resonances are seen to be associated with symmetric collision lifetime eigenchannels, they have significantly different spatial characteristics." @default.
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- W2011794324 date "1988-11-01" @default.
- W2011794324 modified "2023-10-14" @default.
- W2011794324 title "Collision lifetime matrix analysis of the two lowest energy resonances in the collinear H + H2 system" @default.
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- W2011794324 doi "https://doi.org/10.1016/0301-0104(88)87110-6" @default.
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