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• W2011965212 abstract "The complexity of silicate minerals makes prediction of their dissolution rates a challenging problem. A combination of large cluster ab-initio quantum mechanical models and chemical probe dissolution experiments are used to understand the dissolution process for olivine-group minerals. Rapid release of M2+ cations by precursor reactions involving H+ attack at µ3-O surface sites produces a silica-enriched surface. Slower rates of silica release via a ligand exchange reaction involving a proton in the activated complex controls the overall rate of olivine dissolution. Our results provide a physical explanation for the correlation among olivine dissolution rates and water exchange rates for the corresponding aqueous cation." @default.
• W2011965212 created "2016-06-24" @default.
• W2011965212 creator A5082313910 @default.
• W2011965212 date "2006-02-01" @default.
• W2011965212 modified "2023-10-16" @default.
• W2011965212 title "Mechanism for the dissolution of olivine series minerals in acidic solutions" @default.
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• W2011965212 doi "https://doi.org/10.2138/am.2006.2077" @default.
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