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- W2011985909 abstract "Abstract The macroscopic non-liner optical susceptibility X(2) for a system of partially oriented molecules is written as the ensemble average of molecular hyperpolarizability tensors β. The orientational distribution of these molecules is described by a probability function expanded in Wigner matrices. For a rotationally invariant system X(2) has seven non-vanishing components, and a method is outlined to determine these by sum- or difference-frequency mixing experiments. The method could be applied to electrically poled samples, adsorbates liquid crystals and membranes to determine several components of the molecular hyperpolarizability tensor, or to extract information about the orientational distribution." @default.
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- W2011985909 date "1985-06-01" @default.
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- W2011985909 title "Irreducible tensor analysis of sum- and difference-frequency generation in partially oriented samples" @default.
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- W2011985909 doi "https://doi.org/10.1016/0301-0104(85)85085-0" @default.
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