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• W2012040704 abstract "There is increasing evidence that surface plasmons could catalyze photochemical reactions of organic molecules on metal surfaces. However, due to the complex interactions among the substrate, the adsorbate, the environment, and the incident light, the existence and the underlying mechanism of such catalytic processes have been under intense debate. Here we present a systematic first principles study on one of the most studied and controversial systems, namely, p-aminobenzenethiol (PATP) adsorbed on silver nanoparticles. Our calculations have confirmed that the observed surface-enhanced Raman scattering (SERS) bands at 1142, 1391, and 1440 cm–1 of PATP on silver surfaces belong to its coupling reaction product, 4,4′-dimercaptoazobenzene (DMAB). It is found that the deprotonation or protonation of N atoms is the key initial step for the transformations between PATP and DMAB. The photodecomposition reaction from DMAB to PATP can occur only under the conditions that both proton transfer and plasmonic excitati..." @default.
• W2012040704 created "2016-06-24" @default.
• W2012040704 creator A5057282533 @default.
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• W2012040704 creator A5082788658 @default.
• W2012040704 date "2014-03-21" @default.
• W2012040704 modified "2023-10-02" @default.
• W2012040704 title "Roles of Plasmonic Excitation and Protonation on Photoreactions of p-Aminobenzenethiol on Ag Nanoparticles" @default.
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• W2012040704 doi "https://doi.org/10.1021/jp500728s" @default.
• W2012040704 hasPublicationYear "2014" @default.
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