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- W2012055229 abstract "At 300 K the low pressure association reactions of Al+ with C6H6, C6H5D, [1,3,5]-C6H3D3, and C6D6 have been studied by using Fourier transform ion cyclotron resonance (FTICR) mass spectrometry. Several rate constants were found to correlate with the deuterium content of the benzenes. For example, radiative association (kra) correlates with the content of D atoms, ranging from 1.7 × 10−12 (for C6H6) to 6.2 × 10−12 cm3 molecule−1 s−1 (for C6D6). IR photon emission (kr) occurs with a rate constant varying from (17 ± 5) s−1 (C6D6) to (24 ± 7) s−1 (C6H6). Rate constants (kb) for the unimolecular dissociation of the chemically activated collision complexes back to reactants range from (3 ± 1) × 103 s−1 (C6D6) to (16 ± 5) × 103 s−1 (C6H6). Ab initio molecular orbital calculations and equilibrium measurements were used to assess a bond dissociation energy of BDE(Al+−(C6H6)) = 39.0 kcal mol−1, and equilibrium measurements indicate BDE(Al+−(C6D6)) > BDE(Al+(C6H6))." @default.
- W2012055229 created "2016-06-24" @default.
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- W2012055229 date "1995-11-01" @default.
- W2012055229 modified "2023-10-16" @default.
- W2012055229 title "Isotope effects in radiative cooling: the Al(C6H6)+ system" @default.
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- W2012055229 doi "https://doi.org/10.1016/0168-1176(95)04223-8" @default.
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