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• W2012084244 abstract "New hybrid complexes of polypyridyl ruthenium and pyridylporphyrins have been prepared by the coordination of pyridyl nitrogens to the ruthenium centers. A 1:4 hybrid complex, [{Ru(bpy)(trpy)}4(mu4-H2Py4P)]8+ ([1]8+) (bpy = 2,2'-bipyridine; trpy = 2,2':6',2-terpyridine; H2Py4P = 5,10,15,20-tetra(4-pyridyl)porphyrin), has been characterized by the single-crystal X-ray diffraction method. A 1:1 complex, [{Ru(bpy)(trpy)}(H2PyT3P)]2+ ([2]2+) (H2PyT3P = 5-(4-pyridyl)tritolylporphyrin) has also been prepared. The Soret band of the porphyrin ring shifts to longer wavelength with some broadening, the extent of the shift being larger for [1]8+. Cyclic voltammograms of the two complexes show simple overlap of the component redox waves. The complexes are weakly emissive at room temperature, which becomes stronger at lower temperatures. While [1]8+ at >140 K and [2]2+ at 77-280 K show only porphyrin fluorescence, [1]8+ at <140 K shows ruthenium and porphyrin phosphorescence, in addition to the porphyrin fluorescence." @default.
• W2012084244 created "2016-06-24" @default.
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• W2012084244 date "2006-07-27" @default.
• W2012084244 modified "2023-09-28" @default.
• W2012084244 title "Structural, Redox, and Photophysical Studies of the Tetra(pyridyl)porphyrin Complex Containing Four (2,2‘-Bipyridine)(2,2‘:6‘,2‘ ‘-terpyridine)ruthenium(II) Groups" @default.
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• W2012084244 doi "https://doi.org/10.1021/ic0602852" @default.
• W2012084244 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16903745" @default.
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