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- W2012100785 abstract "The hypothesis that S∗ is a vibrationally-excited ground-state population is tested and discarded for two carotenoid samples: β-carotene in solution and rhodopin glucoside embedded in the light harvesting 2 protein from Rhodopseudomonas acidophila. By demonstrating that the transient absorption signals measured in both systems that are induced by broadband (1000 cm−1) and narrowband (50 cm−1) excitation pulses are near identical and hence bandwidth independent, the impulsive stimulated Raman scattering mechanism proposed as the primary source for S∗ generation is discarded. To support this conclusion, previously published multi-pulse pump–dump–probe signals [17] are revisited to discard secondary mechanisms for S∗ formation." @default.
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- W2012100785 date "2010-02-01" @default.
- W2012100785 modified "2023-10-18" @default.
- W2012100785 title "Using narrowband excitation to confirm that the S∗ state in carotenoids is not a vibrationally-excited ground state species" @default.
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- W2012100785 doi "https://doi.org/10.1016/j.cplett.2010.01.014" @default.
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